表面流人工湿地微污染进水下沉积物营养盐累积特征及污染评价
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1.河海大学环境学院;2.河海大学农业科学与工程学院;3.生态环境部南京环境科学研究所;4.盐城市水务集团有限公司

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国家自然科学基金面上项目(522035511)


Accumulation Characteristics and Pollution Assessment of Nutrients in Sediments of Surface Flow Constructed Wetlands Treating Slightly Polluted Water *
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1.College of Environment,Hohai University;2.Yancheng Water Affairs Treatment Co,Ltd

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    摘要:

    本研究旨在探究大型表流人工湿地在长期净化微污染水体过程中,湿地沉积物中碳、氮、磷等的时空分布特征及主要影响因素。为此,采集了盐龙湖28个底泥采样点,测定了样品的有机碳(TOC)、总氮(TN)、总磷(TP)等含量,对沉积物中有机碳、总氮和总磷进行相关性分析,最后对沉积物污染物进行综合污染评价和有机污染评价。研究结果显示,盐龙湖沉积物中TP的平均含量为529 mg/kg,TN的平均含量为953 mg/kg,TOC的平均含量为0.85%。TN、TP呈极显著正相关(r=0.729,P<0.01),TN、TOC呈显著正相关(r=0.251,P<0.05),说明底泥中的有机氮和有机碳可能是相同的来源。①顺水流方向,沉积物TP、TN在各分区有下降趋势,其中预处理区底泥营养盐含量最高,污染也最为严重;②在垂向分布上,盐龙湖各分区底泥营养盐含量有表层富集的特征,含量高值主要集中在0~30 cm。与2017年相比,挺水区底泥营养盐沿水流方向有下降趋势,挺水区沉积物TP和TOC含量大于2017年,主要由于挺水区在运行多年以后,藻类残体、附着在颗粒上的污染物在进水处沉积较多,微生物降解和释放N、P等营养元素。根据综合污染指数法和有机污染指数法评价结果可知,盐龙湖底泥整体质量较好,氮磷污染程度除预处理区为中度污染水平外,其它区域均为清洁或轻度污染水平;有机污染程度除预处理区和深度净化区为轻度污染水平外,其它区域均为清洁水平。研究结果可为大型表流人工湿地在长期运行中的底泥污染评估提供科学参考。

    Abstract:

    This study investigates the spatiotemporal distribution patterns and key influencing factors of carbon, nitrogen, and phosphorus in sediments of a large surface-flow constructed wetland during long-term remediation of slightly polluted water.We collected sediment samples from 28 sites in Yanlong Lake and analyzed the contents of total organic carbon (TOC), total nitrogen (TN), and total phosphorus (TP). Correlation analyses were performed among these parameters, followed by comprehensive pollution and organic pollution assessments. Results revealed average concentrations of 529 mg/kg TP, 953 mg/kg TN, and 0.85% TOC in the sediments. Strong positive correlations were observed between TN and TP (r=0.729, P<0.01) and between TN and TOC (r=0.251, P<0.05), suggesting shared organic sources for nitrogen and carbon. Key spatial patterns emerged: ① Along the water flow direction, TP and TN contents showed decreasing trends across different zones, with the pretreatment area exhibiting the highest nutrient levels and most severe pollution; ② Vertical distribution displayed surface enrichment (0-30 cm) of nutrients across all zones. Compared to 2017 data, the emergent plant zone demonstrated decreasing nutrient trends along flow direction but higher TP and TOC contents, attributable to accumulated algal debris, particle-bound pollutants, and microbial-mediated nutrient release at the inlet area. Pollution assessment using comprehensive and organic pollution indices indicated generally good sediment quality throughout Yanlong Lake. Nitrogen and phosphorus pollution ranged from moderate in the pretreatment zone to clean/mild in other areas, while organic pollution was mild only in pretreatment and advanced treatment zones but clean elsewhere. These findings provide valuable scientific references for sediment pollution evaluation in large surface-flow constructed wetlands during extended operation.

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  • 收稿日期:2025-05-06
  • 最后修改日期:2026-04-04
  • 录用日期:2025-10-10
  • 在线发布日期: 2025-11-20
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